Thursday Jan. 19, 2006

A few remaining sets of Experiment #1 materials were distributed in class.  A couple of handouts that discussed the Donora, Pennsylvania air pollution disaster and SO2 pollution in Russia were distributed in class.

A couple more things concerning increasing carbon dioxide concentrations and its possible effect on climate (you might want to refer back to the last paragraph in the class notes from Jan. 17.

The Keeling curve shows us that the atmospheric CO2 concentration has been increasing since 1958.  What was happening before that?  How can we determine atmospheric concentrations in the past anyways?


Ice has been accumulating in Antarctica and Greenland for hundreds of thousands perhaps millions of years.  The ice sheets are two miles thick in some locations.  As this ice was deposited (in the form of snow) small volumes of the ancient atmosphere were also trapped in bubbles in the ice.  Scientists have drilled into the ice sheets and removing cores of ice.  They have then been able to extract and analyze the gases in the bubbles.  They are actually able to measure CO2 concentrations in past atmospheres.

A small portion of what they have found is shown in the following figure (the top of p. 3 in the photocopied notes).
atmospheric carbon dioxide concentration prior to 1958
The red portion of the graph above shows the Keeling curve measurements that were made starting in 1958.  The green portion shows CO2 concentration measurements based on ice cores.  You can see that CO2 concentration was fairly constant up until 1750 or so.  That is about the time of the start of the "Industrial Revolution."  Burning fossil fuels to power machines and factories began adding larger amounts of CO2 to the atmosphere.

The figure below shows that other greenhouse gases (methane [CH4] and nitrous oxide [N2O]) have also been increasing since the start of the industrial revolution.

increasing concentrations of carbon dioxide, methane, and nitrous oxide
This figure is from "Climate Change 2001: The Scientific Basis," published by the Intergovernmental Panel on Climate Change (www.ipcc.ch).

what has average temperature been doing as the concentration of greenhouse gases has been increasing?
OK if greenhouse gas concentrations have been increasing since about 1750, What has the global average surface temperature been doing during this same time period? The overall change in shown on the bottom part of p. 3 in the photocopied notes.

change in global average surface temperature between 1860 and 1990

This figure doesn't show the average temperature rather how the average temperature has changed over the past 130 or 140 years.  The change is relative to the 1950 to 1980 30-year average (the dotted line).  Between 1860 and about 1920 the global average temperature was about 0.3o C cooler than the 1950 to 1980 average.  The temperature rose between 1920 and 1940.  The 1940 to 1970 section is somewhat puzzling.  The exact cause of this slight cooling is unknown.  Temperatures have increased from 1970 to the present day.  Many scientists think that this second period of warming can be attributed to increasing greenhouse gas concentrations.

Detecting such a small overall change in temperature for the earth is difficult.  Instruments and locations at which measurements were made have changed (imagine how Tucson has changed in the last 130 years or so).  There is also a considerable amount of year to year variation.  About 70% of the earth is covered by oceans and measurements over oceans are more difficult to make.

The graph above was smoothed to show the overall change.  The top figure below shows the actual year to year variation (red bars) and gives you an idea of the uncertainly in the yearly average temperature measurements (black vertical lines).

changes in global average surface temperature
The lower curve shows estimates of global average surface temperature for times before 1860.  This is more difficult.  This is not based on actual measurements of temperature.  We can't directly measure the temperature of the air trapped in the bubbles of polar ice (like can be done with CO2 concentration), the temperature has changed.  Scientists have come up with other techniques to try to indirectly determine temperatures in the past.  We will probably discuss some of this work later in the semester.  [These two figures are also from the Intergovernmental Panel on Climate Change report].


In the remainder of the class today and during the first part of next Tuesday's class we will learn about two more pollutants: tropospheric ozone and carbon monoxide.

stratospheric and tropospheric ozone

Ozone has a kind of "Dr. Jeckell and Mr Hyde personality."  Stratospheric ozone is beneficial because it absorbs dangerous high-energy ultraviolet light.  Tropospheric ozone is bad, it is a pollutant..  It is also a key ingredient in photochemical smog. 

We will try to make some photochemical smog later in a class demonstration.  That will require ozone.  We will make use of the relatively simple stratospheric process for making ozone (see 2 step process above).  As we will see a more complex series of reactions is used in the troposphere.


At this point a small mercury vapor lamp was inserted into a large 4 liter flask.  The lamp emits a lot of ultraviolet radiation and is used to produce ozone inside the flask.  The flask was sealed with foil so that the ozone couldn't escape.  The glass walls of the flask should absorb the dangerous UV radiation.  But just to play it safe the flask was covered with a black cloth.  The ozone will be used later in the class to make photochemical smog.

tropospheric ozone

The production of tropospheric ozone begins with nitric oxide (NO).  NO is produced when nitrogen and oxygen are heated (in an automobile engine for exampe) and react.  The NO can then react with oxygen to make nitrogen dioxide, a poisonous brown-colored gas.  Sunlight can dissociate (split) the nitrogen dioxide molecule producing atomic oxygen (O) and NO.  O and O2 react (just as they do in the stratosphere) to make ozone (O3).  Because ozone does not come directly from an automobile tailpipe or factory chimney, but only shows up after a series of reactions, it is a secondary pollutant.   The nitric oxide would be an example of a primary pollutant.

NO is produced early in the day.  The concentration of NO2 peaks somewhat later.  Peak ozone concentrations are usually found in the afternoon.  Ozone concentrations are also usually higher in the summer than in the winter.  This is because sunlight plays a role in ozone production and summer sunlight is more intense than winter sunlight.
ozone reacts with hydrocarbons to make photochemical smog
Ozone reacts with a hydrocarbon of some kind to make a product gas.  This product gas sometimes condenses to make a visible smog cloud or haze.

The class demonstration of photochemical smog is summarized below.  We begin by using the UV lamp to fill the flask with ozone.  Then a few pieces of fresh lemon peel were added to the flask.  A whitish cloud quickly became visible (colored brown in the figure below).

photochemical smog demonstration


We next briefly discussed the first experiment.  With the experiment materials students instructions concerning the experiment and also the report they will write about the experiment.
experiment #1 setup

The object of Experiment #2 is to measure the percentage oxygen concentration in the air.  A moist piece of steel wool is stuck into a graduated cylinder and the open end of the cylinder is immersed in a cup of water.  Note water won't just enter the cylinder when you try to immerse it.  Air pressure keeps the water out.  You must first insert a piece of flexible tubing into the cylinder (half inside half outside) and then immerse the cylinder.  Lower it until the water level can just be read on the cylinder scale then remove the tubing.  The experiment is underway.

oxygen in the cylinder reacts with steel wool to make rust
Oxygen in the air inside the cylinder will react with the steel wool to make rust.  Oxygen is removed from the air sample.  As this occurs the water level will gradually rise (you should explain in your report why removal of the oxygen causes the water level to change).  Eventually the water level will stop rising, this indicates that all of the oxygen has been used up and that the experiment is over.

carbon monoxide
 
Carbon monoxide (CO) is a colorless, odorless, toxic gas.  It is a primary pollutant that results from incomplete combustion (complete combustion would produce carbon dioxide).  The highest CO concentrations are observed on winter mornings.  CO is trapped in stable morning surface inversion layers.